000 01654nab a2200205 4500
005 20260520000928.0
008 260224s2011 xxu
245 0 0 _aStudies of bitumen-silica and oil-silica interactions in ionic liquids
260 _a
_b
_cene./feb. 2011
270 _a04/04/2011 ; 04/04/2011
300 _a7 p. ; 293–299
520 _aTranscripción del resumen del autor. Previous work in this laboratory has shown that bitumen and oil can be readily separated from sand, using ionic liquids at ambient temperatures. To probe the mechanism underlying the relative ease of separation, atomic force microscopy (AFM) has been used to study interaction forces and adhesion between bitumen surfaces and a silica probe in the presence of liquid media. The energy of adhesion between bitumen samples obtained from both Canadian and U.S. oil sands are approximately an order of magnitude smaller in an ionic liquid medium than in aqueous solution. This behavior was traced to the ability of ionic liquids to form layered charge structures on surfaces. Although interactions between the silica probe and an aged crude oil sample could not be determined, because the probe adhesion to the oil film exceeded the force capacity of the AFM, thermodynamic considerations indicate that the energy of separation of silica from aged oil is also significantly smaller in an ionic liquid medium than in aqueous solution.
581 _a1
773 0 _tEnergy & fuels
_g25
942 _cARTICULO
100 1 _aHogshead, Charles G.
_945051
100 1 _aManias, Evangelos
_945052
100 1 _aWilliams, Phillip
_945053
999 _c174406
_d174406