000 01378nab a2200181 4500
005 20260520000831.0
008 260224s2009 xxu
245 0 0 _aDeep oxidative desulfurization of fuels catalyzed by phosphotungstic acid in ionic liquids at room temperature
260 _a
_b
_cmar./abr. 2009
270 _a2009-08-12 ; 2009-08-12
300 _a4 p. ; 1354-1357
520 _aResúmen del autor: A simplified extraction and catalytic oxidative desulfurization (ECODS) system composed of phosphotungstic acid (H3PW12O40·14H2O), 30% H2O2, and [bmim]BF4 was found suitable for the deep removal of sulfur in model oil. By this desulfurization system dibenzothiophene (DBT), 4,6-dimethyldibenzothiophene (4,6-DMDBT), and benzothiophene (BT) could be effectively removed. Removal of DBT could reach 98.2% at room temperature (30 °C) for 1 h, which was remarkably superior to mere solvent extraction with IL (14.2%) or catalytic oxidation without IL (15.9%). When the reaction temperature increased to 70 °C, treatment of BT, DBT, and 4,6-DMDBT with our ECODS system showed 100% removal of sulfur compounds in 3 h. This desulfurization system could be recycled five times with slight decrease in activity
773 0 _tEnergy & fuels
_g23
942 _cARTICULO
100 1 _aLi, Huaming
_941782
100 1 _aHe, Lining
_941783
999 _c170293
_d170293